Alexander van Geen

and 3 more

The roof and spire of Notre-Dame cathedral in Paris that caught _re and collapsed on April 15, 2019, were covered with 460 tons of lead (Pb). Government reports documented Pb deposition immediately downwind of the cathedral and a 20-fold increase in airborne Pb concentrations at a distance of 50 km in the aftermath. For this study, we collected 100 samples of surface soil from tree pits, parks, and other sites in all directions within 1 km of the cathedral. Concentrations of Pb measured by X-ray uorescence range from 30 to 9000 mg/kg across the area, with a higher proportion of elevated concentrations to the northwest of the cathedral, in the direction of the wind prevailing during the fire. By integrating these observations with a Gaussian process regression model, we estimate that the average concentration of Pb in surface soil downwind of the cathedral is 430 (95% interval, 300-590) mg/kg, nearly double the average Pb concentration in the other directions of 240 (95% interval, 170-320) mg/kg. The di_erence corresponds to an integrated excess Pb inventory within a 1 km radius of 1.0 (95% interval, 0.5-1.5) tons, about 0.2% of all the Pb covering the roof and spire. This is over 6 times the estimated amount of Pb deposited downwind 1-50 km from the cathedral. To what extent the concentrated fallout within 1 km documented here temporarily exposed the downwind population to Pb is di_cult to con_rm independently because too few soil, dust, and blood samples were collected immediately after the fire.